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Synthesis and catalytic activity of histidine-based NHC ruthenium complexes
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| File | Description | Size | Format | |
|---|---|---|---|---|
| DT-001768_manuscript.pdf | 464.01 kB | Adobe PDF | Download |
| Title: | Synthesis and catalytic activity of histidine-based NHC ruthenium complexes | Authors: | Monney, Angèle Venkatachalam, Galmari Albrecht, Martin |
Permanent link: | http://hdl.handle.net/10197/6599 | Date: | 28-Mar-2011 | Abstract: | Main-chain C,N-protected histidine has been successfully alkylated at both side-chain nitrogens. The corresponding histidinium salt was metallated with ruthenium(II) by a transmetalation procedure, thus providing histidine-derived NHC ruthenium complexes. These bio-inspired comsxsxsplexes show appreciable activity in the catalytic transfer hydrogenation of ketones. | Funding Details: | European Research Council | Type of material: | Journal Article | Publisher: | Royal Society of Chemistry | Copyright (published version): | 2011 The Royal Society of Chemistry | Keywords: | Heterocyclic carbene complexes;Transition-metal-complexes;Bioorganometallic chemistry;Amino-acids;Transfer hydrogenation;Asymmetric catalysis;Structural diversity;Directed evolution;Ligands;Reactivity | DOI: | 10.1039/c0dt01768j | Language: | en | Status of Item: | Peer reviewed |
| Appears in Collections: | Chemistry Research Collection |
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